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Evidence for Quaternary climate change in East Africa has been derived from outcrops on land and lake cores and from marine dust, leaf wax, and pollen records. These data have previously been used to evaluate the impact of climate change on hominin evolution, but correlations have proved to be difficult, given poor data continuity and the great distances between marine cores and terrestrial basins where fossil evidence is located. Here, we present continental coring evidence for progressive aridification since about 575 thousand years before present (ka), based on Lake Magadi (Kenya) sediments. This long-term drying trend was interrupted by many wet–dry cycles, with the greatest variability developing during times of high eccentricity-modulated precession. Intense aridification apparent in the Magadi record took place between 525 and 400 ka, with relatively persistent arid conditions after 350 ka and through to the present. Arid conditions in the Magadi Basin coincide with the Mid-Brunhes Event and overlap with mammalian extinctions in the South Kenya Rift between 500 and 400 ka. The 525 to 400 ka arid phase developed in the South Kenya Rift between the period when the last Acheulean tools are reported (at about 500 ka) and before the appearance of Middle Stone Age artifacts (by about 320 ka). Our data suggest that increasing Middle- to Late-Pleistocene aridification and environmental variability may have been drivers in the physical and cultural evolution ofHomo sapiensin East Africa.

Saline alkaline lakes that precipitate sodium carbonate evaporites are most common in volcanic terrains in semi‐arid environments. Processes that lead to trona precipitation are poorly understood compared to those in sulphate‐dominated and chloride‐dominated lake brines. Nasikie Engida (Little Magadi) in the southern Kenya Rift shows the initial stages of soda evaporite formation. This small shallow (<2 m deep; 7 km long) lake is recharged by alkaline hot springs and seasonal runoff but unlike neighbouring Lake Magadi is perennial. This study aims to understand modern sedimentary and geochemical processes in Nasikie Engida and to assess the importance of geothermal fluids in evaporite formation. Perennial hot‐spring inflow waters along the northern shoreline evaporate and become saturated with respect to nahcolite and trona, which precipitate in the southern part of the lake, up to 6 km from the hot springs. Nahcolite (NaHCO₃) forms bladed crystals that nucleate on the lake floor. Trona (Na₂CO₃·NaHCO₃·2H₂O) precipitates from more concentrated brines as rafts and as bottom‐nucleated shrubs of acicular crystals that coalesce laterally to form bedded trona. Many processes modify the fluid composition as it evolves. Silica is removed as gels and by early diagenetic reactions and diatoms. Sulphate is depleted by bacterial reduction. Potassium and chloride, of moderate concentration, remain conservative in the brine. Clastic sedimentation is relatively minor because of the predominant hydrothermal inflow. Nahcolite precipitates when and wherepCO₂is high, notably near sublacustrine spring discharge. Results from Nasikie Engida show that hot spring discharge has maintained the lake for at least 2 kyr, and that the evaporite formation is strongly influenced by local discharge of carbon dioxide. Brine evolution and evaporite deposition at Nasikie Engida help to explain conditions under which ancient sodium carbonate evaporites formed, including those in other East African rift basins, the Eocene Green River Formation (western USA), and elsewhere.

Many previous studies on lacustrine basins in the East African Rift System have directed their attention to climatic controls on contemporary sedimentation or climate change as part of palaeoenvironmental reconstruction. In contrast, this research focuses on the impact of tectonism and volcanism on rift deposition and develops models that help to explain their roles and relative importance. The study focuses on the spatial and temporal variability in bulk sediment geochemistry from a diverse range of modern and ancient rift sediments through an analysis of 519 samples and 50 major and trace elements. The basins examined variously include, or have contained, wetlands and/or shallow to deep, fresh to hypersaline lakes. Substantial spatial variability is documented for Holocene to modern deposits in lakes Turkana, Baringo, Bogoria, Magadi and Malawi. Mio‐Pleistocene sediments in the Central Kenya Rift and Quaternary deposits of the southern Kenya Rift illustrate temporal variability. Tectonic and volcanic controls on geochemical variability are explained in terms of: (i) primary controlling factors (faulting, subsidence, uplift, volcanism, magma evolution and antecedent lithologies and landscapes); (ii) secondary controls (bedrock types, rift shoulder and axis elevations, accommodation space, meteoric and hydrothermal fluids and mantleCO₂); and (iii) response factors (catchment area size, orographic rains, rain shadows, vegetation densities, erosion and weathering rates, and spring/runoff ratios). The models developed have, in turn, important implications for palaeoenvironmental interpretation in other depositional basins.